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Teacher of Chemistry Teacher of Chemical & Biomolecular Engineering 211 Lewis Hall (510) 642-0860 (510) 642-8369 209 Lewis (510) 643-3832 Research Competence and Interest Inorganic and materials chemistry; synthesis of inorganic particles and higher dimensional solids; accurate customizing of chemical and physical properties; gas storage, molecular separations, and catalysis in permeable materials; magnetic and conductive products.

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We utilize a variety of physical techniques to analyze and define our products thoroughly, including by gas adsorption analysis, X-ray and neutron diffraction, various spectroscopic techniques, and SQUID magnetometry. To learn more about the Long group and a complete list of publications, please go to the group site. Metal, Organic Frameworks A significant focus of research study in the Long group is the style and study of metalorganic frameworksporous, inorganic solids developed of metal nodes connected by natural linkersthat are of interest for applications varying from gas storage and molecular separations to catalysis and battery applications.

In addition, now more than ever international warming is demanding a remarkable reduction in our global greenhouse emissions. One of the most promising short-term emissions mitigation strategiesand therefore an important separations needis the elimination of CO2 directly from the flue gas streams of coal- and natural gas-fired power plants. Toward this end, we are studying a brand-new class of diamine-appended structures established in our group that show high CO2 separation capabilities in the existence of water, with minimal energy requirements arising from an unprecedented cooperative adsorption system.

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We are also targeting metalorganic structures featuring polarizing open metal websites and shape-discriminating pore structures for the boosted binding of H2 and CH4 near ambient temperatures and the separation of hydrocarbon isomers, respectively. The high-capacity storage of hydrogen and gas is particularly relevant for automobile transportation, as these gases represent promising cleaner alternatives to liquid hydrocarbon fuels, and yet significant advances in adsorbent innovations are required to overcome the pricey restrictions currently imposed by low-temperature and high-pressure on-board storage requirements.

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Catalysis and Conductivity In addition to their function as molecular screens, metalorganic structures are guaranteeing as robust, efficient drivers with isolated and distinct active websites. We are looking for to utilize coordinatively-unsaturated framework metal centers as catalytic websites and likewise setting up these metal centers post-synthetically by means of chelating groups built into the structure ligands.