The natural splendour of the Park's rugged mountains, with its waters and vegetation, offer particular places of great interest and beauty.
Towns of particular interest, from a historical point of view, are Bagà, being once the capital of the Barony of Pinós, and Bellver de Cerdanya centre of an ancient batllia (mayorship).
There are a good number of towns that still keep their traditional and rural architecture such as Castellar de n'Hug. Other towns of equal interest and beauty are Saldes, with its castle ruins, and Montellà, Tuixén, Josa de Cadí, not to mention other smaller villages and hamlets such as Torres d'Alàs, Adraén, el Quer Foradat, Cornellana, Cava, Ansovell, Gisclareny, Gréixer and Gósol (where Picasso painted interesting works in 1906).